To return something which has been crumpled, closer to its original state.
I took the wadded up letter from the trash and carefully uncrumpled it.
(intransitive) Having been crumpled, to return closer to one's original state.
As the newspaper uncrumpled, the picture on the frontpage become recognizable.
Origin of Uncrumple
un- + crumple
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Words Starting With U and Ending With E